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The fact that HEMs can be tailored by compositional design, among others, makes them so exciting and versatile. This typically leads to strong interactions between the incorporated elements, so-called cocktail effects, and in some cases, to an entropy stabilization. In general, HEMs rely on the high-entropy concept, that is, the introduction of a large number of elements in a single-phase structure to increase the configurational entropy 5. Lately, a new class of multicomponent ceramics, high-entropy materials (HEMs), is receiving attention for rechargeable lithium-ion battery (LIB) applications 1, 2, 3, 4. Overall, the data confirm that the AE technology as a non-destructive operando technique holds promise for gaining insight into the degradation processes occurring in battery cells during cycling. In the subsequent cycles, AE was mainly detected during delithiation, a finding we attribute to the progressive crack formation and propagation. The initial cycle was found to be the most acoustically active because of solid-electrolyte interphase formation and chemo-mechanical degradation. Especially the clustering of AE signals allows for correlations of acoustic events with various processes. Here, we probe the conversion-type HEO material in lithium half-cells by acoustic emission (AE) monitoring. Because high-entropy oxides constitute a new class of electrode materials, systematic understanding of their behavior during ion insertion and extraction is yet to be established. Among them, the rocksalt (Co 0.2Cu 0.2Mg 0.2Ni 0.2Zn 0.2)O (HEO) has been shown to be a promising high-capacity anode material. What's New: Includes important security enhancements - reccomended for all new and existing users ! Includes OCR.In recent years, high-entropy oxides are receiving increasing attention for electrochemical energy-storage applications.
#Pdf xchange viewer 2.5 196 pdf#
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